High-Curie-temperature ferromagnetism in self-organized Ge(1-x)Mn(x) nanocolumns.

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High-Curie-temperature ferromagnetism in self-organized Ge(1-x)Mn(x) nanocolumns.

Nat Mater. 2006 Jul 9;

Authors: Jamet M, Barski A, Devillers T, Poydenot V, Dujardin R, Bayle-Guillemaud P, Rothman J, Bellet-Amalric E, Marty A, Cibert J, Mattana R, Tatarenko S

The emerging field of spintronics would be dramatically boosted if room-temperature ferromagnetism could be added to semiconductor nanostructures that are compatible with silicon technology. Here, we report a high-TC (>400K) ferromagnetic phase of (Ge,Mn) epitaxial layer. The manganese content is 6%, and careful structural and chemical analyses show that the Mn distribution is strongly inhomogeneous: we observe eutectoid growth of well-defined Mn-rich nanocolumns surrounded by a Mn-poor matrix. The average diameter of these nanocolumns is 3nm and their spacing is 10nm. Their composition is close to Ge(2)Mn, which corresponds to an unknown germanium-rich phase, and they have a uniaxially elongated diamond structure. Their Curie temperature is higher than 400K. Magnetotransport reveals a pronounced anomalous Hall effect up to room temperature. A giant positive magnetoresistance is measured from 7,000% at 30K to 200% at 300K and 9T, with no evidence of saturation.

PMID: 16845420 [PubMed - as supplied by publisher]

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